There's many series that I want to watch (Baccano for example) but won't because I feel like I'm missing out by not having read the visual novel it was based on.
Small correction: Baccano was a series of LIGHT novels (which are basically just books lol).
I haven't personally read them but from what i understand it was a pretty faithful adaptation and incredibly enjoyable in its own right. the light novels do continue after the point where the anime stops, but i do think the anime can stand on its own pretty well.
also if you want to see something with good fleshed out characters, try paranoia agent.
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