Yeah, enemies no longer drop Mythrils or Orichalcums. You have to manually grind the materials for them.
Mythrils require Mythril Shard x5 and Mythril Stone x 2 if I'm not mistaken.
And 3 Mystery Goos, if memory serves me right. Also, Orichalcums can now be bought from Huey, Louie, and Dewey after rescuing Kairi from Hollow Bastion. Each costs 5,000 munny.
Anyway… I really don't think there's anything that can be done. Pretty much the synthesis progression has come to a halt, and from what the OP described, there's no way to move forward. SeruOmen, if you're still aiming for that Master Synthesis trophy, I think your best bet is to do it on a new playthrough.
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